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Super-resolving single nitrogen vacancy centers within single nanodiamonds using a localization microscope.

Gu M, Cao Y, Castelletto S, Kouskousis B, Li X

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  • Journal Optics express

  • Published 07 Apr 2014

  • Volume 21

  • ISSUE 15

  • Pagination 17639-46

  • DOI 10.1364/OE.21.017639

Abstract

In this paper, we show super-resolving single nitrogen vacancy (NV) centers with a sub-20 nanometer resolution in a wide-field localization microscope based on the discovery of photoluminescence blinking in high-pressure high-temperature nanodiamonds (NDs). The photon statistics reveals that NDs containing not only single but also multiple NV centers show photoluminescence blinking. The combination of an atomic force microscope and an optical localization microscope built on the blinking feature enables the optically resolved two NV centers within single NDs for the first time. Our method establishes new avenues for studying nanoscale photon dynamics associated with single NV centers within NDs together with ND-based ultra-sensitive bioimaging devices.